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      KCI등재 SCOPUS SCIE

      Highly efficient electroluminescence devices with a mixed layer of SnO2 and colloidal quantum dots

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      https://www.riss.kr/link?id=A108281450

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      다국어 초록 (Multilingual Abstract)

      We demonstrate the high efficiency of quantum dot light-emitting diodes (QLEDs) that consist of amixed layer of SnO2 nanoparticles (NPs) and quantum dots (QDs). A stable mixture of SnO2 NPs andQDs is prepared in chlorobenzene and then applied to QLEDs with no separate electron transportlayer (ETL). QLEDs with such a simplified structure produce a maximum luminance of 142,855 cd/m2,an EQE of 9.42%, and a current efficiency of 41.18 cd/A that result from the improved charge balanceof the mixed layer. This produces one of the best device performances of QLEDs with a non-ZnO inorganicETL, clearly indicating the remarkable promise of using SnO2 NPs as an inorganic ETL for QLEDs.
      Moreover, the reduction of fabrication steps in this solution-based process proves advantageous tonext-generation display technology.
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      We demonstrate the high efficiency of quantum dot light-emitting diodes (QLEDs) that consist of amixed layer of SnO2 nanoparticles (NPs) and quantum dots (QDs). A stable mixture of SnO2 NPs andQDs is prepared in chlorobenzene and then applied to QLEDs...

      We demonstrate the high efficiency of quantum dot light-emitting diodes (QLEDs) that consist of amixed layer of SnO2 nanoparticles (NPs) and quantum dots (QDs). A stable mixture of SnO2 NPs andQDs is prepared in chlorobenzene and then applied to QLEDs with no separate electron transportlayer (ETL). QLEDs with such a simplified structure produce a maximum luminance of 142,855 cd/m2,an EQE of 9.42%, and a current efficiency of 41.18 cd/A that result from the improved charge balanceof the mixed layer. This produces one of the best device performances of QLEDs with a non-ZnO inorganicETL, clearly indicating the remarkable promise of using SnO2 NPs as an inorganic ETL for QLEDs.
      Moreover, the reduction of fabrication steps in this solution-based process proves advantageous tonext-generation display technology.

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      참고문헌 (Reference)

      1 L. Qian, "Stable and efficient quantum-dot light-emitting diodes based on solution-processed multilayer structures" 5 : 543-548, 2011

      2 H. Moon, "Stability of quantum dots, quantum dots films, and quantum dot light-emitting diodes for display applications" 31 : 1804294-, 2019

      3 J. Bahadur, "Solution processed Mo doped SnO2as an effective ETL in the fabrication of low temperature planer perovskite solar cell under ambient conditions" 67 : 159-167, 2019

      4 Y. Liu, "Quantum-sized SnO2 nanoparticles with upshifted conduction band: a promising electron transportation material for quantum dot light-emitting diodes" 36 : 6605-6609, 2020

      5 D. Sun, "Purification and stabilization of colloidal ZnO nanoparticles in methanol" 43 : 237-243, 2007

      6 D.Cao, "Preparation of ZnO nanoparticles with high dispersibility based on oriented attachment (OA) process" 14 : 210-, 2019

      7 S. N. Vijayaraghavan, "Low-temperature processed highly efficient hole transport layer free carbon-based planar perovskite solar cells with SnO2 quantum dot electron transport layer" 13 : 100204-, 2020

      8 V.L. Colvin, "Lightemitting diodes made from cadmium selenide nanocrystals and a semiconducting polymer" 370 : 354-357, 1994

      9 S. Coe, "Large-area ordered quantum-dotmonolayers via phase separation during spin-casting" 15 : 1117-1124, 2005

      10 Z. Xu, "La-doped SnO2 as ETL for efficient planarstructure hybrid perovskite solar cells" 73 : 62-68, 2019

      1 L. Qian, "Stable and efficient quantum-dot light-emitting diodes based on solution-processed multilayer structures" 5 : 543-548, 2011

      2 H. Moon, "Stability of quantum dots, quantum dots films, and quantum dot light-emitting diodes for display applications" 31 : 1804294-, 2019

      3 J. Bahadur, "Solution processed Mo doped SnO2as an effective ETL in the fabrication of low temperature planer perovskite solar cell under ambient conditions" 67 : 159-167, 2019

      4 Y. Liu, "Quantum-sized SnO2 nanoparticles with upshifted conduction band: a promising electron transportation material for quantum dot light-emitting diodes" 36 : 6605-6609, 2020

      5 D. Sun, "Purification and stabilization of colloidal ZnO nanoparticles in methanol" 43 : 237-243, 2007

      6 D.Cao, "Preparation of ZnO nanoparticles with high dispersibility based on oriented attachment (OA) process" 14 : 210-, 2019

      7 S. N. Vijayaraghavan, "Low-temperature processed highly efficient hole transport layer free carbon-based planar perovskite solar cells with SnO2 quantum dot electron transport layer" 13 : 100204-, 2020

      8 V.L. Colvin, "Lightemitting diodes made from cadmium selenide nanocrystals and a semiconducting polymer" 370 : 354-357, 1994

      9 S. Coe, "Large-area ordered quantum-dotmonolayers via phase separation during spin-casting" 15 : 1117-1124, 2005

      10 Z. Xu, "La-doped SnO2 as ETL for efficient planarstructure hybrid perovskite solar cells" 73 : 62-68, 2019

      11 G. Motomura, "Improvement of electroluminescent characteristics in quantum dot lightemitting diodes using ZnInP/ZnSe/ZnS quantum dots by mixing an electron transport material into the lightemitting layer" 10 : 065228-, 2020

      12 H. Lee, "Improved efficiency of inverted organic light-emitting diodes using tin dioxide nanoparticles as an electron injection layer" 5 : 1977-1981, 2013

      13 J. Zhou, "Ideal CdSe/CdS core/shell nanocrystals enabled by entropic ligands and their core size-, shell thickness-, and liganddependent photoluminescence properties" 139 : 16556-16567, 2017

      14 K. H. Lee, "Highly efficient, colorreproducible full-color electroluminescent devices based on red/green/blue quantum dot-mixed multilayer" 9 : 10941-10949, 2015

      15 J. Xu, "High-performance blue quantumdot light emitting diode via solvent optimization strategy for ZnO nanoparticles" 11 (11): 959-, 2021

      16 B. S. Mashford, "High-efficiency quantum-dot light-emitting devices with enhanced charge injection" 7 : 407-412, 2013

      17 Q. Chen, "Gate-tunable all-inorganic QLED with enhanced charge injection balance" 8 : 1280-1285, 2020

      18 N. Kirkwood, "Enhancing quantum dot LED efficiency by tuning electron mobility in the ZnO electron transport layer" 3 : 1600868-, 2016

      19 H. Zhang, "Efficient red/green/blue tandem quantum-dot light-emitting diodes with external quantum efficiency exceeding 21%" 12 : 697-704, 2018

      20 M. Park, "Colloidal quantumdot light-emitting diodesemploying solution-processable tin dioxide nanoparticles in an electron transport layer" 10 : 8261-8265, 2020

      21 H. Liu, "A facile room temperature solution synthesis of SnO2 quantum dots for perovskite solar cells" A7 : 10636-10643, 2019

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