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Park, Y. I.,Postupna, O.,Zhugayevych, A.,Shin, H.,Park, Y.-S.,Kim, B.,Yen, H.-J.,Cheruku, P.,Martinez, J. S.,Park, J. W.,Tretiak, S.,Wang, H.-L. Royal Society of Chemistry 2015 Chemical Science Vol.6 No.1
<▼1><P>Fabrication of a unique white light LED from a stimuli-responsive organic molecule is reported. Emission properties are dominated by the pH of the solution through intermolecular charge transfer.</P></▼1><▼2><P>A new, pH dependent and water-soluble, conjugated oligomer (amino, trimethylammonium oligophenylene vinylene, <B>ATAOPV</B>) was synthesized with a quaternary ammonium salt and an aromatic amine at the two ends of a π-conjugated oligomer, thus creating a strong dipole across the molecule. A unique white light LED is successfully fabricated from a stimuli responsive organic molecule whose emission properties are dominated by the pH value of the solution through controlled intermolecular charge transfer.</P></▼2>