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Hong Thi Bich Truong,Hiep Nghia Bui,Hieu Trung Nguyen,Thanh-Luu Pham,Duy Ngoc Nguyen,Yuan-Shing Perng,Linh Thi My Lam,Thi-Dieu-Hien Vo,Van-Truc Nguyen,Ha Manh Bui 한국화학공학회 2022 Korean Journal of Chemical Engineering Vol.39 No.4
Electron-beam (EB) irradiation was employed to degrade enrofloxacin (ENR) in an aqueous solution. Thealgal growth inhibition test revealed that ENR exhibited low toxicity against the cyanobacterium Arthrospira sp., with anEC50-96 h value of 5.17mg/L. The Taguchi design also involved finding the best optimum for ENR treatment using EB. Results revealed that the high-efficiency removal of ENR in an aqueous solution was approximately 98.53% under theoptimum conditions of an absorbed dose of 5 kGy, a pH of 5.0, and an initial ENR concentration of 10 mg/L and anH2O2 concentration of 2mM. The ERR degradation under a couple of EB irradiation and H2O2 followed pseudo-firstorderkinetics, with an R2 of ~0.970. The major degradation pathways of ENR were suggested by density functional theory,natural bond orbital calculations, and liquid chromatography-tandem mass spectrometry (LC/MS/MS) analysis. Lifecycle assessment (LCA) was also performed to evaluate the impact of the EB on removing ENR; the industrial processwas designed based on laboratory tests aimed with the ReCiPe tool. The obtained results indicated that energy consumptionand H2O2 affect environmental impacts with order human health, ecology systems, and natural resource. The LCAalso proved that EB could be a green and efficient method for eliminating pharmaceutical contaminants in water.