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Nurdin Muhammad,Watoni Abdul Haris,Natsir Muhammad,Rahmatilah Sarifa,Maulidiyah Maulidiyah,Wibowo Dwiprayogo,Salim La Ode Agus,Sadikin Siti Naqiyah,Bijang Catherina Manukpadang,Umar Akrajas Ali 한국화학공학회 2023 Korean Journal of Chemical Engineering Vol.40 No.9
The modification of ternary metal oxide to improve the photoelectrocatalysis (PEC) properties of TiO2 photocatalyst is a hot issue in environmental and resource applications. Herein, we present a novel photoelectrocatalytst of Se doped-TiO2/Ti nanotube arrays (Se@TiO2/Ti-NTAs) for high-efficiency degradation of diazinon pesticide. The Se@TiO2/Ti-NTAs were prepared to treat the TiO2-NTAs in Se-TiO2 sol-gel for 10 min, which was followed by calcination in air at 200 °C for 1 h. Optical absorption spectroscopy of the Se@TiO2/Ti-NTAs indicated that there is a red-shift in the optical energy gap to 2.95 eV if compared to the pristine TiO2/Ti NTAs, which suggests that the new photoelectrocatalyst is photoactive under visible light irradiation. We evaluated the photoactivity of the sample by using it as the photoelectrocatalyst in the degradation of diazinon pesticides under the PEC process. The results showed that the Se@TiO2/Ti-NTAs can degrade 95.62% for 1 h under visible light irradiation, which is equivalent to the degradation rate constant of 0.0183 s−1. For comparison, the pristine TiO2/Ti NTAs only degrades the diazinon as high as 87.65%, even then under UV light irradiation. Our result also indicated that the Se@TiO2/Ti-NTAs promote active photoelectron transfer and active radical formation, such as •OH and •O − 2 , for rapid diazinon pesticide degradation. The Se@TiO2/Ti-NTAs photoelectrode should be a potential platform for environmental pollution treatment.
Nanocomposite design of graphene modified TiO2 for electrochemical sensing in phenol detection
Muhammad Nurdin,Maulidiyah Maulidiyah,Abdul Haris Watoni,Armawansa Armawansa,La Ode Agus Salim,Zul Arham,Dwiprayogo Wibowo,Irwan Irwan,Akrajas Ali Umar 한국화학공학회 2022 Korean Journal of Chemical Engineering Vol.39 No.1
This study is the stage of developing a phenol detection electrochemical sensor. Phenol is one of the organic pollutants harmful to human life and ecosystems. The development of this sensor was carried out by studying the use of TiO2 anatase as a modifier of graphene electrodes. The mass of TiO2 anatase was varied, while the mass of graphene and paraffin was fixed. The results showed that the TiO2 mass of 1.0 g was the best mass as a graphene electrode modifier. The use of this mass increases the oxidation current (Ipa) of phenol by 450 A, which is observed at an oxidation potential (Epa) of −0.30 V. The presence of interfering ions such as K+, Fe2+, and OH− can decrease the measurement current. However, based on the %RSD value, it shows that the performance of TiO2-graphene is in a good category, where the %RSD value obtained is 0.6%. TiO2-graphene electrodes can be used repeatedly for 12 days. Overall, this work demonstrates the potential of TiO2-graphene electrodes as electrode candidates for electrochemical-based phenol sensors.