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RISS 인기검색어
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- 저자 : Shenyu (검색결과 3 건)
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Steering Coacervation by a Pair of Broad-Spectrum Regulators
Yang, Shenyu,Li, Bo,Wu, Chunxian,Xu, Weiwei,Tu, Mei,Yan, Yun,Huang, Jianbin,Drechsler, Markus,Granick, Steve,Jiang, Lingxiang American Chemical Society 2019 ACS NANO Vol.13 No.2
<P>Coacervation is liquid-liquid phase separation ubiquitous in industrial applications and cellular biology. Inspired by cellular manipulation of coacervate droplets such as P granules, we report here a regulatory strategy to manipulate synthetic coacervation in a spatiotemporally controllable manner. Two oppositely charged small molecules are shown to phase separate into coacervate droplets in water as a result of electrostatic attraction, hydrophobic effect, and entropy. We identify a down regulator, β-cyclodextrin, to disrupt the hydrophobic effect, thus dissolving the droplets, and an up regulator, amylase, to decompose β-cyclodextrin, thus restoring the droplets. The regulation kinetics is followed in real time on a single-droplet level, revealing diffusion-limited dissolution and reaction-limited condensation, respectively, taking ∼4 s and 2-3 min. Versatility of this strategy to manipulate the coacervation is demonstrated in two aspects: spatially distributed coacervation in virtue of amylase-grafted hydrogel frameworks and coacervate transportation across membranes and hydrogel networks <I>via</I> a disassemble-to-pass strategy. The current regulatory pairs and strategies are anticipated to be general for a wide variety of synthetic self-assembly systems.</P> [FIG OMISSION]</BR>
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First-principles analysis of the absorption and luminescence properties of Cr2+-doped ZnSe crystal
Yuqin Zhang,Guoying Feng,Shenyu Dai,Shougui Ning,Shouhuan Zhou 한국물리학회 2016 Current Applied Physics Vol.16 No.5
The electronic band structure, absorption and luminescence properties of Cr2+-doped ZnSe crystal have been investigated by first-principles calculations on the basis of density functional theory. Firstprinciples calculations were carried out using the Vienna Ab-initio Simulation Package (VASP). It is shown that isolated impurity bands that mainly made up of Cr(d) orbitals are created in the band gap with the doping of Cr2+ ions. The Cr(d) orbitals are split into e and t2 groups because of the potential of the crystal. Theoretical absorption and luminescence spectra are calculated and compared with experimental data. An appropriate explanation of the experimental spectra is presented.
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Yi-Kai Zeng,Shenyu Bo,Jun-hui Wang,Bin Cui,Lei Zhu,Won-Chun Oh,Hao Gu 한국재료학회 2020 한국재료학회지 Vol.30 No.11
In this work, Ag3PO4/In2S3 nanocomposites with low loading of In2S3 (5-15 wt %) are fabricated by two step chemical precipitation approach. The microstructure, composition and improved photoelectrochemical properties of the asprepared composites are studied by X-ray diffraction pattern (XRD), field emission scanning electron microscopy (SEM), transmission electron microscopy (TEM), X-ray photoelectron spectroscopy (XPS), photocurrent density, EIS and amperometric i-t curve analysis. It is found that most of In2S3 nanoparticles are deposited on the surfaces of Ag3PO4. The as-prepared Ag3PO4/ In2S3 composite (10 wt%) is selected and investigated by SEM and TEM, which exhibits special morphology consisting of lager size substrate (Ag3PO4), particles and some nanosheets (In2S3). The introduction of In2S3 is effective at improving the charge separation and transfer efficiency of Ag3PO4/In2S3, resulting in an enhancement of photoelectric behavior. The origin of the enhanced photoelectrochemical activity of the In2S3-modified Ag3PO4 may be due to the improved charge separation, photocurrent stability and oriented electrons transport pathways in environment and energy applications.
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