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Efficient solar-light photocatalytic H2 evolution of Mn0.5Cd0.5S coupling with S,N-codoped carbon
Hao Peng,Congying Huang,Xiaogang Zheng,Jing Wen 한국공업화학회 2022 Journal of Industrial and Engineering Chemistry Vol.106 No.-
The low-cost and highly-efficient photocatalysts for solar-light induced water splitting had drawn greatattention to develop the renewable hydrogen economy. To enhance the solar-light driven H2 evolution ofMn0.5Cd0.5S, Mn0.5Cd0.5S was modified by S,N-codoped carbon (3-MCS/SN-C) via the in-situ sulfurizationat high temperature. In contrast with Mn0.5Cd0.5S (11.13 mmol g1 h1) and S-doped g-C3N4(0.35 mmol g1 h1), the optimal 3-MCS/SN-C with a mass ratio of Mn0.5Cd0.5S to S,N-codoped carbonof 1:3 exhibited the best H2 evolution rate of 27.58 mmol g1 h1 and an apparent quantum yield of27.43% at 400 nm. The photo-corrosion induced to the decreased H2 evolution capacity of 3-MCS/SN-Cfrom 131.13 to 126.52 mmol g1 after five cycles of 5 h. S,N-codoped carbon could efficiently capture visiblelight and absorb the photons, leading to the efficient transformation and separation of photogeneratedcarriers at the junction interface between Mn0.5Cd0.5S and S,N-codoped carbon.
Lu Li,Congying Shao,Qian Wu,Yunjian Wang,Mingzhu Liu 성균관대학교(자연과학캠퍼스) 성균나노과학기술원 2018 NANO Vol.13 No.12
In this work, water-soluble and blue-emitting carbon nanodots (CDs) were synthesized from apple peels for the first time via one-step hydrothermal method. The synthetic route is facile, green, economical and viable. The as-prepared CDs were characterized thoroughly by transmission electron microscopy (TEM), X-ray diffraction (XRD), Raman, Fourier transform infrared (FT-IR), X-ray photoelectron (XPS), fluorescence and UV–Vis absorption spectroscopy in terms of their morphology, surface functional groups and optical properties. The results show that these CDs possessed ultrasmall size, good dispersivity, and high tolerance to pH, ionic strength and continuous UV irradiation. Significantly, the CDs had fast and reversible response towards temperature, and the accurate linear relationship between fluorescence intensity and temperature was used to design a novel nanothermometer in a broad temperature range from 5 to 65 ℃ facilely. In addition, the fluorescence intensity of CDs was observed to be quenched immediately by Cr(VI) ions based on the inner filter effect. A low-cost Cr(VI) ions sensor was proposed employing CDs as fluorescent probe, and it displayed a wide linear range from 0.5 to 200 μM with a detection limit of 0.73 μM. The practicability of the developed Cr(VI) sensor for real water sample assay was also validated with satisfactory recoveries.
Xiaogang Zheng,Fuyan Kang,Congying Huang,Sihao Lv,JinYang Zhang,Hao Peng 한국공업화학회 2020 Journal of Industrial and Engineering Chemistry Vol.88 No.-
ZnS–ZnO–Sm2O3 (Zn–Sm–XY) composites were prepared via the high-temperature calcination of coreshellstructured ZnS@Sm2O3 for the enhanced photocatalytic degradation of dyes and antibiotics invisible light region. Effects of calcined temperature, Sm2O3 content, pH value, contaminantconcentration, and inorganic ions on the photocatalytic activity were investigated. Ternary Zn–Smcomposites exhibit the excellent photocatalytic activity for the visible light driven degradation oftetracycline hydrochloride. Among these composites, Zn–Sm–2B prepared via the heat-treatment ofZnS–Sm2O3 at 673 K shows the best photocatalytic activity for the removal of tetracycline hydrochloride. The enhanced photocatalytic activity of Zn–Sm–2B is also achieved for the visible light drivendegradation of methyl orange, methylene blue, and rhodamine B within 20 min. In addition, Zn–Sm–6Ccalcined from Zn–Sm–C at 1073 K as well as Zn–Sm–2B exhibits excellent photocatalytic activity. OH andO2radicals are vital for the enhanced photocatalytic activity of Zn–Sm–2B and Zn–Sm–2B in visiblelight region, respectively. The lattice defects, sulfur vacancies, and oxygen vacancies facilitate the efficientcharge transfer and the rapid separation of electron-hole pairs at the junction interface of Zn–Sm–2B.
Xuefeng Zhong,Shuai Che,Congying Xie,Lan Wu,Xinyu Zhang,Lin Tian,Chan Liu,Hongbo Li,Guoying Du The Korean Society of Phycology 2023 ALGAE Vol.38 No.2
Light quality is a common environmental factor which influences the metabolism of biochemical substances in algae and leads to the response of algal growth and development. Pyropia yezoensis is a kind of economic macroalgae that naturally grows in the intertidal zone where the light environment changes dramatically. In the present study, P. yezoensis thalli were treated under white light (control) and monochromatic lights with primary colors (blue, green, and red) for 14 days to explore their physiological response to light quality. During the first 3 days of treatment, P. yezoensis grew faster under blue light than other light qualities. In the next 11 days, it showed better adaptation to green light, with higher growth rate and photosynthetic capacity (reflected by a higher rETR<sub>max</sub> = 61.58 and E<sub>k</sub> = 237.78). A higher non-photochemical quenching was observed in the treatment of red light than others for 14 days. Furthermore, the response of P. yezoensis to light quality also results in the difference of photosynthetic pigment contents. The monochromatic light could reduce the synthesis of all pigments, but the reduction degree was different, which may relate to the spectral absorption characteristics of pigments. It was speculated that P. yezoensis adapted to a specific or changing light environments by regulating the synthesis of pigments to achieve the best use of light energy in photosynthesis and premium growth and metabolism.
Analyzing behavior of circular concrete-filled steel tube column using improved fuzzy models
Yuxin Zheng,Hongwei Jin,Congying Jian,Zohre Moradi,Mohamed Amine Khadimallah,Hossein Moayedi 국제구조공학회 2022 Steel and Composite Structures, An International J Vol.43 No.5
Axial compression capacity (Pu) is a significant yet complex parameter of concrete-filled steel tube (CFST) columns. This study offers a novel ensemble tool, adaptive neuro-fuzzy inference system (ANFIS) supervised by equilibrium optimization (EO), for accurately predicting this parameter. Moreover, grey wolf optimization (GWO) and Harris hawk optimizer (HHO) are considered as comparative supervisors. The used data is taken from earlier literature provided by finite element analysis. ANFIS is trained by several population sizes of the EO, GWO, and HHO to detect the best configurations. At a glance, the results showed the competency of such ensembles for learning and reproducing the Pu behavior. In details, respective mean absolute errors along with correlation values of 4.1809% and 0.99564, 10.5947% and 0.98006, and 4.8947% and 0.99462 obtained for the EO-ANFIS, GWO-ANFIS, and HHO-ANFIS, respectively, indicated that the proposed EO-ANFIS can analyze and predict the behavior of CFST columns with the highest accuracy. Considering both time and accuracy, the EO provides the most efficient optimization of ANFIS and can be a nice substitute for experimental approaches.
Ying Ma,Yueyan Liu,Congying Deng,Xiang Chen,Yang Zhao,Sheng Lu,Youqi Wang 한국섬유공학회 2020 Fibers and polymers Vol.21 No.10
3-D woven textile is generated through the weaving process. Yarn is a non-continuum material domain, thestructure of which is determined by inter fiber movement. In this study, the micro-geometry of 3-D orthogonal weave isgenerated at filament level predicting through the weaving process implementing the digital element approach (DEA). First,the basic concepts and explicit algorithm of DEA is introduced. The method of calculating adjusted digital fiber materialproperty in terms of discretization resolution is proposed. Second, the unit-cell topology of 3-D orthogonal weave is definedby a position matrix. The calculation of potential energy of the cell is derived. At last, a dynamic weaving process is designedto investigate the effect of yarn tension on fabric micro-geometry and cell energy. 4 unit-cells are generated under 4 sets oftension combination. Results show that as the fabric thickness decrease, the filaments of the weft yarns move towards thecenter. The weft yarns at the top and bottom deform into their final shape first. The applied tension on weaver plays adominant role in determining fabric thickness and convergence speed. By comparing the numerical results with themicroscope pictures taken from the actual specimen, it is concluded that the fabric micro-geometry produced by tensioncombination 4 closely matches the experimental results.
Zheng, Yuxin,Jin, Hongwei,Jiang, Congying Techno-Press 2022 Advances in nano research Vol.13 No.2
In this paper, a finite element (FE) simulation has been developed in order to examine the nonlinear stability of reinforced sandwich beams with graphene oxide powders (GOPs). In this regard, the nonlinear stability curves have been obtained asuming that the beam is under compressive loads leading to its buckling. The beam is considered to be a three-layered sandwich beam with metal core and GOP reinforced face sheets and it is rested on elastic substrate. Moreover, a higher-order refined beam theory has been considered to formulate the sandwich beam by employing the geometrically perfect and imperfect beam configurations. In the solving procedure, the utalized finite element simulation contains a novel beam element in which shear deformation has been included. The calculated stability curves of GOP-reinforced sandwich beams are shown to be dependent on different parameters such as GOP amount, face sheet thickness, geometrical imperfection and also center deflection.