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Le Floc'h, V.,Brasselet, S.,Zyss, J.,Cho, B. R.,Lee, S. H.,Jeon, S.-J.,Cho, M.,Min, K. S.,Suh, M. P. WILEY-VCH Verlag 2005 Advanced Materials Vol.17 No.2
<B>Graphic Abstract</B> <P>An octupolar crystal is produced from octupolar molecules of 1,3,5-tricyano-2,4,6-tris(p-diethylaminostyryl)benzene and its structure is elucidated experimentally using the combined polarization analysis of two-photon fluorescence and second-harmonic generation (SHG). The optimal crystalline packing of the molecules in the crystal (which originates from intermolecular &pgr;–&pgr; stacking interactions)—see Figure—results in a large SHG efficiency. <img src='wiley_img/09359648-2005-17-2-ADMA200400451-content.gif' alt='wiley_img/09359648-2005-17-2-ADMA200400451-content'> </P>