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      저자 : Farzaneh Feyzi (검색결과 2 건)
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        Four phase hydrate equilibria of methane and carbon dioxide with heavy hydrate former compounds: Experimental measurements and thermodynamic modeling

        Farzaneh Feyzi,Hamed Tavasoli 한국화학공학회 2016 Korean Journal of Chemical Engineering Vol.33 No.8

        We experimentally investigated the hydrate dissociation condition for four phase hydrate (H)-aqueous liquid (LAq)-hydrocarbon rich liquid (LHC)-vapor (V) for the ternary systems of help gas-heavy hydrate former-water. Methane and carbon dioxide are known as help gases and benzene and cyclohexane are considered as heavy hydrate formers. The experimental data were generated using an isochoric pressure-search method. Two different equations of state (EOS) were employed to study the equilibrium phase behavior of ternary four phase systems. The EOSs considered are Valderama-Patel-Teja EOS combined with non-density dependent mixing rule (VPT+NDD) and Statistical Associating Fluid Theory EOS proposed by Huang and Radosz (SAFT-HR). The required binary interaction parameters (BIP) were obtained using vapor-liquid equilibrium (VLE) and liquid-liquid equilibrium (LLE) data. The hydrate phase was modeled by the modification of the solid solution theory of van der Waals and Platteeuw. To obtain reliable results, distortion of cages due to occupation of large molecules was considered. The Kihara parameters of cyclohexane were adjusted to hydrate dissociation data. Model calculations for hydrate forming conditions were found to be in satisfactory agreement with the newly reported data in this work and literature data.

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        Development of electrolyte SAFT-HR equation of state for single electrolyte solutions

        Azam Najafloo,Farzaneh Feyzi,Ali Taghi Zoghi 한국화학공학회 2014 Korean Journal of Chemical Engineering Vol.31 No.12

        The explicit version of the mean spherical approximation (MSA) is added to the SAFT-HR equation ofstate (EoS) to model aqueous alkali halide solutions. The proposed electrolyte equation of state (eEoS) has two par-ameters per each ion. Two methods are in common use for calculating ion parameters: ion-based and salt-based. Inthis work, the electrolyte parameters are obtained for 61 single electrolyte solutions using salt-based method. Usingthis approach, mean ionic activity coefficients of the 61 aqueous electrolyte systems were modeled with overall averageabsolute relative percent deviation (AAD%) of 3.91. Also, for testing the ability of the model in terms of ionic par-ameters, six salts (NaCl, NaBr, NaI, KCl, KBr and KI) were studied using ion-based method. The liquid densities, os-motic coefficients and salt mean ionic activity coefficients of 6 aqueous electrolyte solutions were modeled with overallAAD% of 0.68, 2.28 and 0.96, respectively.

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